Excitons in strain-induced one-dimensional moiré potentials at transition metal dichalcogenide heterojunctions

Yusong Bai, Lin Zhou, Jue Wang, Wenjing Wu, Leo J. McGilly, Dorri Halbertal, Chiu Fan Bowen Lo, Fang Liu, Jenny Ardelean, Pasqual Rivera, Nathan R. Finney, Xu Chen Yang, D. N. Basov, Wang Yao, Xiaodong Xu, James Hone, Abhay N. Pasupathy*, X. Y. Zhu*

*Corresponding author for this work

Research output: Contribution to journalJournal Articlepeer-review

Abstract

The possibility of confining interlayer excitons in interfacial moiré patterns has recently gained attention as a strategy to form ordered arrays of zero-dimensional quantum emitters and topological superlattices in transition metal dichalcogenide heterostructures. Strain is expected to play an important role in the modulation of the moiré potential landscape, tuning the array of quantum dot-like zero-dimensional traps into parallel stripes of one-dimensional quantum wires. Here, we present real-space imaging of unstrained zero-dimensional and strain-induced one-dimensional moiré patterns along with photoluminescence measurements of the corresponding excitonic emission from WSe2/MoSe2 heterobilayers. Whereas excitons in zero-dimensional moiré traps display quantum emitter-like sharp photoluminescence peaks with circular polarization, the photoluminescence emission from excitons in one-dimensional moiré potentials shows linear polarization and two orders of magnitude higher intensity. These results establish strain engineering as an effective method to tailor moiré potentials and their optoelectronic response on demand.

Original languageEnglish
Pages (from-to)1068-1073
Number of pages6
JournalNature Materials
Volume19
Issue number10
DOIs
Publication statusPublished - 1 Oct 2020
Externally publishedYes

Bibliographical note

Publisher Copyright:
© 2020, The Author(s), under exclusive licence to Springer Nature Limited.

Fingerprint

Dive into the research topics of 'Excitons in strain-induced one-dimensional moiré potentials at transition metal dichalcogenide heterojunctions'. Together they form a unique fingerprint.

Cite this