Abstract
A theory for impulsive resonant pump-probe and photon-echo spectroscopies of polyatomic dyes in solution is developed. A multimode calculation in which the intramolecular and solvation modes are modeled as Brownian oscillators is presented. Electronic dephasing, the time-dependent Stokes shift, and quantum beats are analyzed.
| Original language | English |
|---|---|
| Pages (from-to) | 6920-6923 |
| Number of pages | 4 |
| Journal | Physical Review A - Atomic, Molecular, and Optical Physics |
| Volume | 42 |
| Issue number | 11 |
| Publication status | Published - 1990 |
| Externally published | Yes |
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