TY - JOUR
T1 - Near-Infrared Mobile Cloud OA-ICOS Sensor System for Atmospheric Carbon Dioxide Monitoring
AU - Zhang, Lei
AU - Hua, Ying
AU - Zhou, Yishen
AU - Zheng, Kaiyuan
AU - Song, Fang
AU - Chang, Zhiyong
AU - Zheng, Chuantao
N1 - Publisher Copyright:
© 2025 American Chemical Society.
PY - 2025/2/25
Y1 - 2025/2/25
N2 - Based on near-infrared off-axis integrated cavity output spectroscopy (OA-ICOS), a portable carbon dioxide (CO2) sensor system capable of atmosphere monitoring is proposed by targeting the CO2 absorption lines at 2.004 μm. To address the comprehensive issues of complex light-adjustment structures, poor sealing, and slow gas replacement, an effective optimization scheme is introduced, combining fluid dynamics to produce a stable optical resonant cavity with an optical path length of 891 m and a physical length of 30 cm. The sensor system boasts a wide dynamic range of 0.011-800 parts per million (ppm), with a limit of detection (LoD) of 11 parts per billion (ppb) at an averaging time of 0.5 s. To address the issues of long monitoring time and cumbersome data supervision, a cloud monitoring system was developed based on a master control module, a cloud server, and a portable monitoring terminal. Field mobile monitoring of urban CO2 was conducted over a large area in Changchun city, along with a 7-day fixed-point detection on the campus of Jilin University, verifying the reliability and application potential of the mobile CO2 monitoring system in field applications.
AB - Based on near-infrared off-axis integrated cavity output spectroscopy (OA-ICOS), a portable carbon dioxide (CO2) sensor system capable of atmosphere monitoring is proposed by targeting the CO2 absorption lines at 2.004 μm. To address the comprehensive issues of complex light-adjustment structures, poor sealing, and slow gas replacement, an effective optimization scheme is introduced, combining fluid dynamics to produce a stable optical resonant cavity with an optical path length of 891 m and a physical length of 30 cm. The sensor system boasts a wide dynamic range of 0.011-800 parts per million (ppm), with a limit of detection (LoD) of 11 parts per billion (ppb) at an averaging time of 0.5 s. To address the issues of long monitoring time and cumbersome data supervision, a cloud monitoring system was developed based on a master control module, a cloud server, and a portable monitoring terminal. Field mobile monitoring of urban CO2 was conducted over a large area in Changchun city, along with a 7-day fixed-point detection on the campus of Jilin University, verifying the reliability and application potential of the mobile CO2 monitoring system in field applications.
UR - https://www.webofscience.com/wos/woscc/full-record/WOS:001420585500001
UR - https://openalex.org/W4407398536
UR - https://www.scopus.com/pages/publications/85217535580
M3 - Journal Article
SN - 0003-2700
VL - 97
SP - 4021
EP - 4030
JO - Analytical Chemistry
JF - Analytical Chemistry
IS - 7
ER -