Photoinduced phase transitions by time-resolved far-infrared spectroscopy in V2O3

M. K. Liu*, B. Pardo, J. Zhang, M. M. Qazilbash, Sun Jin Yun, Z. Fei, Jun Hwan Shin, Hyun Tak Kim, D. N. Basov, R. D. Averitt

*Corresponding author for this work

Research output: Contribution to journalJournal Articlepeer-review

55 Citations (Scopus)

Abstract

Using time-resolved far-infrared spectroscopy, we observe multiple routes for photoinduced phase transitions in V2O3. This includes (i)a photothermal antiferromagnetic to paramagnetic transition and (ii)an incipient strain-generated paramagnetic metal to paramagnetic insulator transition, which manifests as coherent oscillations in the far-infrared conductivity. The ∼100ps conductivity oscillation results from coherent acoustic phonon modulation of the bandwidth W. Our results indicate that poor metals are particularly amenable to coherent strain control of their electronic properties.

Original languageEnglish
Article number066403
JournalPhysical Review Letters
Volume107
Issue number6
DOIs
Publication statusPublished - 3 Aug 2011
Externally publishedYes

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